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dc.contributor.authorParlett, CMA
dc.contributor.authorArandiyan, H
dc.contributor.authorDurndell, Lee
dc.contributor.authorIsaacs, MA
dc.contributor.authorLopez, AT
dc.contributor.authorWong, RJ
dc.contributor.authorWilson, K
dc.contributor.authorLee, AF
dc.date.accessioned2022-09-05T10:48:06Z
dc.date.available2022-09-05T10:48:06Z
dc.date.issued2022-01
dc.identifier.issn1387-1811
dc.identifier.issn1873-3093
dc.identifier.other111535
dc.identifier.urihttp://hdl.handle.net/10026.1/19598
dc.description.abstract

Ordered mesoporous silicas are widely used in separation science and catalysis, however, their slow batch synthesis is a barrier to scale-up and new applications. SBA-15 is one of the most extensively studied and commercially available mesoporous silicas, whose textural properties can be readily tuned through judicious choice of synthesis conditions. Here we demonstrate the continuous flow synthesis of SBA-15 in high yield at 80 °C using a simple tube reactor without any mixing device. The resulting SBA-15 exhibits excellent textural properties, with a BET surface area of 566 m2 g−1 and ordered 5.1 nm mesopore channels in a p6mm arrangement, akin to those from conventional batch synthesis, but with far higher productivity than previously reported in batch or flow (5.3 g L−1 h−1 versus 0.4 and 0.6 g L−1 h−1 respectively).

dc.format.extent111535-111535
dc.languageen
dc.language.isoen
dc.publisherElsevier BV
dc.rightsAttribution-NonCommercial-NoDerivatives 4.0 International
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
dc.subjectMesoporous silica
dc.subjectContinuous flow
dc.subjectSBA-15
dc.subjectMaterial synthesis
dc.titleContinuous-flow synthesis of mesoporous SBA-15
dc.typejournal-article
dc.typeJournal Article
plymouth.author-urlhttps://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000722319700005&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=11bb513d99f797142bcfeffcc58ea008
plymouth.volume329
plymouth.publication-statusPublished
plymouth.journalMicroporous and Mesoporous Materials
dc.identifier.doi10.1016/j.micromeso.2021.111535
plymouth.organisational-group/Plymouth
plymouth.organisational-group/Plymouth/Faculty of Science and Engineering
plymouth.organisational-group/Plymouth/Faculty of Science and Engineering/School of Geography, Earth and Environmental Sciences
plymouth.organisational-group/Plymouth/REF 2021 Researchers by UoA
plymouth.organisational-group/Plymouth/REF 2021 Researchers by UoA/UoA12 Engineering
plymouth.organisational-group/Plymouth/Users by role
plymouth.organisational-group/Plymouth/Users by role/Academics
dcterms.dateAccepted2021-10-27
dc.identifier.eissn1873-3093
dc.rights.embargoperiodNot known
rioxxterms.versionofrecord10.1016/j.micromeso.2021.111535
rioxxterms.licenseref.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
rioxxterms.typeJournal Article/Review


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